Optical rotation quasi-phase-matching for circularly polarized high harmonic generation

Quantum-classical correspondence in circularly polarized high harmonic generation

Circularly polarized molecular high harmonic generation using a bicircular laser

We investigate the process of circularly polarized high harmonic generation in molecules using a bicircular laser field. In this context, we show that molecules offer a very robust framework for the production of circularly polarized harmonics, provided their symmetry is compatible with that of the laser field. Using a discrete time-dependent symmetry analysis, we show how all the features (har...

Helicity-selective phase-matching and quasi-phase matching of circularly polarized high-order harmonics: towards chiral attosecond pulses

Phase matching of circularly polarized high-order harmonics driven by counter-rotating bichromatic lasers was recently predicted theoretically and demonstrated experimentally. In that work, phase matching was analyzed by assuming that the total energy, spin angular momentum and linear momentum of the photons participating in the process are conserved. Here we propose a new perspective on phase ...

Quasi-periodic and random quasi-phase matching of high harmonic generation.

Quasi-phase matching schemes employing quasi-periodic or random spatial modulations, previously applied to perturbative nonlinear optics, are demonstrated theoretically for the extreme nonlinear optical process of high harmonic generation. We show that quasi-periodic quasi-phase matching of high harmonic generation can be used for simultaneous enhancement of arbitrarily chosen spectral regions....

High-Efficiency Broadband High-Harmonic Generation from a Single Quasi-Phase-Matching Nonlinear Crystal.

Nonlinear frequency conversion offers an effective way to expand the laser wavelength range based on birefringence phase matching (BPM) or quasi-phase-matching (QPM) techniques in nonlinear crystals. So far, efficient high-harmonic generation is enabled only via multiple cascaded crystals because of the extreme difficulty to simultaneously satisfy BPM or QPM for multiple nonlinear up-conversion...